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• W2069452080 endingPage "3437" @default.
• W2069452080 startingPage "3433" @default.
• W2069452080 abstract "The high-energy deep-core-level spectra of ${mathrm{PrO}}_{2}$ have been studied. Pr 3d x-ray photoemission spectroscopy (XPS), Pr ${M}_{4}$,5 x-ray-absorption spectroscopy (XAS) and Pr ${L}_{3}$ XAS show many-body effects. The data are analyzed in the framework of the filled-band Anderson-impurity model. Starting from the many-body description of the ground-state, the final states of each core-level spectroscopy are predicted. The effective relaxation energy in the final state decreases going from 3d XPS to ${L}_{3}$ XAS to ${M}_{4}$,5 XAS because of the repulsive interaction between the excited electron and the 4f electron in XAS spectra. It is shown that the ground state exhibits mixing of many-body configurations 4${f}^{1}$ and 4${f}^{2}$L, where L denotes a hole in the oxygen 2p-derived valence band, separated by the energy ensuremath{Delta}E=0.5 eV. A nonzero probability of the occupation of the 4${f}^{2}$L configuration, giving a noninteger 4f count ${n}_{f}$=1.6, is found." @default.
• W2069452080 created "2016-06-24" @default.
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• W2069452080 date "1988-08-15" @default.
• W2069452080 modified "2023-09-27" @default.
• W2069452080 title "Many-body effects in praesodymium core-level spectroscopies of<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=normal>PrO</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>" @default.
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• W2069452080 doi "https://doi.org/10.1103/physrevb.38.3433" @default.
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• W2069452080 hasPublicationYear "1988" @default.
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