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• W2069575538 endingPage "R13437" @default.
• W2069575538 startingPage "R13434" @default.
• W2069575538 abstract "Infrared spectroscopy and ab initio quantum chemical cluster calculations are used to study the decomposition of water on the clean $mathrm{Si}(100)ensuremath{-}(2ifmmodetimeselsetexttimesfi{}1)$ surface at low temperature. Using this combined approach we are able to show that the initial surface is actually comprised of an array of isolated and intra-row coupled dimers. The latter are coupled by a hydrogen bonding interaction between OH groups that reside on the same end of adjacent dimers in a dimer row. We find that this interdimer bonding is ensuremath{sim}2 kcal/mol more stable than the isolated dimer case. These findings are postulated to have a significant effect on subsequent oxygen agglomeration." @default.
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• W2069575538 date "1998-11-15" @default.
• W2069575538 modified "2023-10-03" @default.
• W2069575538 title "Heterogeneous nucleation of oxygen on silicon: Hydroxyl-mediated interdimer coupling on<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mi mathvariant=normal>Si</mml:mi><mml:mn /><mml:mo>(</mml:mo><mml:mn>100</mml:mn><mml:mo>)</mml:mo><mml:mo>−</mml:mo><mml:mo>(</mml:mo><mml:mn>2</mml:mn><mml:mn /><mml:mo>×</mml:mo><mml:mn>1</mml:mn><mml:mo>)</mml:mo></mml:math>" @default.
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• W2069575538 doi "https://doi.org/10.1103/physrevb.58.r13434" @default.
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