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• W2069668492 endingPage "R52" @default.
• W2069668492 startingPage "R33" @default.
• W2069668492 abstract "Copper oxide superconductors possess multi-layered structures with a layer sequence of -CuO2 -(Q-CuO2 )n -1 -AO-(MO1± )m -AO- or -CuO2 -B-(O2 -B)s -1 -CuO2 -AO-(MO1± )m -AO- along the elongated caxis. Based on this layer sequence, the known copper oxide structures are categorized as members of the homologous series, Mm Ar Qn -1 Cun Om +r +2n ± (M-mr (n -1)n ; category A) or Mm A2k Bs Cu1+k Om +4k +2s ± (M-m (2k )s (1+k ); category B). Stabilization of such structures especially in the case of high values of the n /sparameter, i.e. the higher members of the homologous series, has been demonstrated to be apparently promoted under high pressures and/or strongly oxidizing conditions. Consequently, techniques for applying both high oxygen gas pressures (10-2000 atm) and ultra-high solid-medium pressures (2-8 GPa) have been advantageously utilized in synthesizing various superconductive copper oxide phases. Especially the ultra-high solid-medium pressure synthesis carried out in the so-called cubic-anvil/belt-type apparatus has proven to be extremely successful in synthesizing novel superconductive phases. In order to achieve high partial pressures of oxygen in the solid-medium environment, `external' oxygen-generating oxides such as KClO4 , KClO3and Ag2 O2are commonly added to the precursor mixtures. It is emphasized that in some cases it is possible to utilize `internal' oxidizing agents alone, i.e. highly oxidized precursors such as BaCuO2+ and Ba2 Cu3 O5+ containing metal constituents common with the desired copper oxide phase only. In the present paper, the potential and applications of high-pressure techniques in synthesizing multi-layered copper oxides and related structures are reviewed and discussed with emphasis on the important `historical' discoveries of novel phases and the present status of controlled production of high-quality samples of such phases." @default.
• W2069668492 created "2016-06-24" @default.
• W2069668492 creator A5076467655 @default.
• W2069668492 creator A5086628462 @default.
• W2069668492 date "2000-03-29" @default.
• W2069668492 modified "2023-10-02" @default.
• W2069668492 title "Application of high-pressure techniques: stabilization and oxidation-state control of novel superconductive and related multi-layered copper oxides" @default.
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