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• W2069878539 endingPage "4080" @default.
• W2069878539 startingPage "4071" @default.
• W2069878539 abstract "To elucidate the nature of processes involved in electrically driven particle aggregation in steady fields, flows near a charged spherical colloidal particle next to an electrode were studied. Electrical body forces in diffuse layers near the electrode and the particle surface drive an axisymmetric flow with two components. One is electroosmotic flow (EOF) driven by the action of the applied field on the equilibrium diffuse charge layer near the particle. The other is electrohydrodynamic (EHD) flow arising from the action of the applied field on charge induced in the electrode polarization layer. The EOF component is proportional to the current density and the particle surface (zeta) potential, whereas our scaling analysis shows that the EHD component scales as the product of the current density and applied potential. Under certain conditions, both flows are directed toward the particle, and a superposition of flows from two nearby particles provides a mechanism for aggregation. Analytical calculations of the two flow fields in the limits of infinitesimal double layers and slowly varying current indicate that the EOF and EHD flow are of comparable magnitude near the particle whereas in the far field the EHD flow along the electrode is predominant. Moreover, the dependence of EHD flow on the applied potential provides a possible explanation for the increased variability in aggregation velocities observed at higher field strengths." @default.
• W2069878539 created "2016-06-24" @default.
• W2069878539 creator A5002712073 @default.
• W2069878539 creator A5022215367 @default.
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• W2069878539 date "2007-03-01" @default.
• W2069878539 modified "2023-10-15" @default.
• W2069878539 title "Electrically Driven Flow near a Colloidal Particle Close to an Electrode with a Faradaic Current" @default.
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• W2069878539 doi "https://doi.org/10.1021/la062870l" @default.
• W2069878539 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/17335253" @default.
• W2069878539 hasPublicationYear "2007" @default.
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