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• W2069883025 startingPage "5863" @default.
• W2069883025 abstract "On-site excitations of the Gd3+ ion in lanthanum ethylsulphate have recently been shown to produce a spin-correlated crystal field which results in zero-field splittings of the same sign as those from experiment but, approximately, two time too large. In this paper intersite one-electron excitations have been invoked to produce additional contributions to the spin-correlated crystal field, which compensate the zero-field splittings from on-site contributions alone to produced zero-field splittings in good agreement with experiment. The resultant zero-field splittings are thus a delicate balance between a number of on-site mechanisms, i.e. a contribution from the paramagnetic Gd3+ ion itself and one from the host in which it is embedded." @default.
• W2069883025 created "2016-06-24" @default.
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• W2069883025 date "1986-10-20" @default.
• W2069883025 modified "2023-10-14" @default.
• W2069883025 title "Inter site contributions to correlated crystal fields and zero-field splittings for Gd3+in lanthanum ethylsulphates" @default.
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• W2069883025 doi "https://doi.org/10.1088/0022-3719/19/29/010" @default.
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