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• W2070169175 abstract "The rotational spectrum of cis-cis HOONO has been studied over a broad range of frequencies, 13–840 GHz, using pulsed beam Fourier-transform microwave spectroscopy and room-temperature flow cell submillimeter spectroscopy. The rotational spectrum of the deuterated isotopomer, cis-cis DOONO, has been studied over a subset of this range, 84–640 GHz. Improved spectroscopic constants have been determined for HOONO, and the DOONO spectrum is analyzed for the first time. Weak-field Stark effect measurements in the region of 84–110 GHz have been employed to determine the molecular dipole moments of cis-cis HOONO [μa=0.542(8)D,μb=0.918(15)D,μ=1.07(2)D] and DOONO [μa=0.517(9)D,μb=0.930(15)D,μ=1.06(2)D]. The quadrupole coupling tensor in the principal inertial axis system for the N14 nucleus has been determined to be χaa=1.4907(25)MHz,χbb=−4.5990(59)MHz,χab=3.17(147)MHz, and χcc=3.1082(59)MHz. Coordinates of the H atom in the center-of-mass frame have been determined with use of the Kraitchman equations, ∣aH∣=0.516Å and ∣bH∣=1.171Å. The inertial defects of HOONO and DOONO are consistent with a planar equilibrium structure with significant out-of-plane H atom torsional motion. Comparisons of the present results are made to ab initio calculations." @default.
• W2070169175 created "2016-06-24" @default.
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• W2070169175 date "2006-02-22" @default.
• W2070169175 modified "2023-10-02" @default.
• W2070169175 title "Rotational spectroscopy and dipole moment of <i>cis-cis</i> HOONO and DOONO" @default.
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• W2070169175 doi "https://doi.org/10.1063/1.2163341" @default.
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