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- W2070667607 abstract "Abstract Using a sol–gel technique, new copper‐functionalised, calcium‐based CO 2 sorbents were developed to integrate chemical looping combustion into the calcium looping scheme. In this process, the exothermic reduction of copper oxide with methane, carbon monoxide or hydrogen is used to provide the heat required to calcine (regenerate) calcium carbonate. The materials contained CuO and CaO in a molar ratio of either 1.3:1 or 3.3:1, were supported on Al 2 O 3 , MgO or MgAl 2 O 4 and were characterised by means of X‐ray diffraction, N 2 physisorption, scanning electron microscopy and temperature‐programmed reduction. All materials, independent of the precursors and support material used, possessed excellent cyclic oxygen‐carrying capacities. However, it was found that the presence of magnesium in the support stabilised the CO 2 uptake and minimised carbon deposition. CuCa‐MgAl‐1.3:1 was the material that possessed the highest CO 2 uptake of 0.13 g g material −1 after 15 cycles of repeated carbonation/calcination–redox reactions." @default.
- W2070667607 created "2016-06-24" @default.
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- W2070667607 date "2012-10-30" @default.
- W2070667607 modified "2023-10-10" @default.
- W2070667607 title "Sol-Gel-Derived, Calcium-Based, Copper-Functionalised CO<sub>2</sub>Sorbents for an Integrated Chemical Looping Combustion-Calcium Looping CO<sub>2</sub>Capture Process" @default.
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- W2070667607 doi "https://doi.org/10.1002/cplu.201200232" @default.
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