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- W2070754476 abstract "The solubility of HCl in cold H 2 SO 4 /H 2 O solutions is central to an assessment of the role of stratospheric aerosol in polar ozone destruction. The interpretation of laboratory measurements of HCl uptake by aqueous H 2 SO 4 requires a knowledge of (1) HCl solubility and (2) the HCl liquid phase diffusion coefficient. Neither quantity is easily determined because of the high H 2 SO 4 concentration and low temperature of the solutions, making experimental data difficult to evaluate and to apply to the real stratospheric situation. To avoid these difficulties, we have used a new thermodynamic model for an improved estimate of HCl solubility, and a viscosity‐based cubic cell model to obtain the diffusion coefficient. The calculated HCl solubility in aqueous H 2 SO 4 below 200 K is up to three orders of magnitude greater than previously thought. This might promote chlorine activation particularly during volcanically perturbed periods with an enhanced stratospheric aerosol loading." @default.
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- W2070754476 date "1994-01-01" @default.
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- W2070754476 title "HCL solubility and liquid diffusion in aqueous sulfuric acid under stratospheric conditions" @default.
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- W2070754476 doi "https://doi.org/10.1029/93gl02956" @default.
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