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• W2070949086 abstract "Abstract The novel nickel-based catalysts with a nickel content of 12 wt% were prepared with the zirconia-alumina composite as the supports. The new carriers, ZrO 2 improved alumina, were synthesized by three methods, i.e., impregnation-precipitation, co-precipitation, and impregnation method. The catalytic properties of these catalysts were investigated in the methanation of carbon dioxide, and the samples were characterized by X-ray diffraction (XRD), X-ray photoelectron spectroscope (XPS), temperature-programmed reduction (TPR) and temperature-programmed desorption (TPD) techniques. The new catalysts showed higher catalytic activity and better stability than Ni/γ-Al 2 O 3 . Furthermore, as a support for new nickel catalyst, the ZrO 2 -Al 2 O 3 composite prepared by the impregnation-precipitation method was more efficient than the other supports in the methanation of carbon dioxide. The highly dispersed zirconium oxide on the surface of γ-Al 2 O 3 inhibited the formation of nickel aluminate-like phase, which was responsible for the better dispersion of Ni species and easier reduction of NiO species, leading to the enhanced catalytic performance of corresponding catalyst." @default.
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• W2070949086 date "2011-05-01" @default.
• W2070949086 modified "2023-10-13" @default.
• W2070949086 title "Methanation of carbon dioxide on Ni/ZrO2-Al2O3 catalysts: Effects of ZrO2 promoter and preparation method of novel ZrO2-Al2O3 carrier" @default.
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• W2070949086 doi "https://doi.org/10.1016/s1003-9953(10)60187-9" @default.
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