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• W2071001498 abstract "A detailed theory is developed for the effects of covalency on the magnetic properties of a Co 2+ ion surrounded by a regular octahedron of ligands. In contrast to previous studies of the cobalt ion, the strong-field representation has been used, in which the octahedral field is diagonalized before the electrostatic interactions. Expressions are derived for the orbital contribution to the g value, and for the ligand hyperfine interactions, in terms of the ligand wave function admixture coefficients. The theory is applied to the electron spin resonance measurements on a Co 2+ : KMgF 3 crystal. In the usual notation the covalent bonding fractions are f σ = 2.9±1.0%, f π = 1.9∓1.0%, f s = 0.54±0.03%, ½( f σ + f π ) = 2.4±0.3%. These results are compared with the results of other authors on different iron group ions." @default.
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• W2071001498 date "1965-02-23" @default.
• W2071001498 modified "2023-09-26" @default.
• W2071001498 title "Concerning the magnetic properties of covalent octahedral cobalt complexes" @default.
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• W2071001498 doi "https://doi.org/10.1098/rspa.1965.0062" @default.
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