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- W2071304330 abstract "Heteroleptic copper(II) complexes were synthesized from three different meso-substituted pyridyl- and quinoline-dipyrrinato ligands (3-pyrdpm, 3-quindpm, and 4-quindpm). Metal complexes were prepared with both acetylacetonate (acac) and hexafluoroacetylactonate (hfacac) ancillary ligands. The complexes undergo a self-complementary self-assembly process upon crystallization to generate a range of solid-state topologies including one-dimensional coordination polymers and discrete hexameric rings. The self-assembly of these molecular aggregates is driven by metal−ligand bonding, but is also modulated by fluorine−fluorine interactions. Perfluorination of the spectator ligand tends to generate more compact structures, which is attributed to aggregation of the perfluoromethyl groups. The results presented here demonstrate that fluorine−fluorine contacts can be used to modulate supramolecular structures in the solid state." @default.
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- W2071304330 date "2005-05-14" @default.
- W2071304330 modified "2023-09-25" @default.
- W2071304330 title "Self-Assembly of Heteroleptic [Cu(dipyrrinato)(hfacac)] Complexes Directed by Fluorine−Fluorine Interactions" @default.
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- W2071304330 doi "https://doi.org/10.1021/ic0504442" @default.
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