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• W2071330488 abstract "A comprehensive kinetic model based on the concept of remote control and today's knowledge of HDS catalysts is developed. It includes the kinetic mechanism of spill-over hydrogen, the creation of active sites by spill-over hydrogen and the catalytic HDS reaction on the created active sites. The HDS rate equations derived here consider both the generation of active sites and the catalytic reactions. The model predictions reproduce the maximum in activity observed in the HDS of thiophene for a certain ratio of Co/Mo in the catalyst. The effect of some physical parameters of the catalyst, which depend upon its preparation and pretreatment, are also investigated. The influence of the hydrogen sulfide to hydrogen ratio is simulated for various Co/Mo ratios in the catalyst. According to the model, multiplicity of steady states would be possible under certain conditions." @default.
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• W2071330488 date "1991-01-01" @default.
• W2071330488 modified "2023-10-18" @default.
• W2071330488 title "Rate equations for the modeling of the synergy in multicomponent catalysts with interconversion of active sites" @default.
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• W2071330488 doi "https://doi.org/10.1016/0009-2509(91)85020-x" @default.
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