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- W2071398413 abstract "Herein, we report a high-yield click synthesis and self-assembly of conjugated amphiphilic block copolymers of polythiophene (PHT) and polyethylene glycol (PEG) and their superstructures. A series of different length PHTm-b-PEGn with well-defined relative block lengths was synthesized by a click-coupling reaction and self-assembled into uniform and stably suspended nanofibers in selective solvents. The length of nanofibers was controllable by varying the relative block lengths while keeping other dimensions and optical properties unaffected for a broad range of fPHT (0.41 to 0.82), which indicates that the packing of PHT dominates the self-assembly of PHTm-b-PEGn. Furthermore, superstructures of bundled and branched nanofibers were fabricated through the self-assembly of PHTm-b-PEGn and preformed PHT nanofibers. The shape, length, and density of the hierarchical assembly structures can be controlled by varying the solvent quality, polymer lengths, and block copolymer/homopolymer ratio. This work demonstrates that complex superstructures of organic semiconductors can be fabricated through the bottom-up approach using preformed nanofibers as building blocks." @default.
- W2071398413 created "2016-06-24" @default.
- W2071398413 creator A5028920276 @default.
- W2071398413 creator A5031867024 @default.
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- W2071398413 date "2012-03-07" @default.
- W2071398413 modified "2023-10-14" @default.
- W2071398413 title "Hierarchical Self-Assembly of Amphiphilic Semiconducting Polymers into Isolated, Bundled, and Branched Nanofibers" @default.
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- W2071398413 doi "https://doi.org/10.1021/nn300385p" @default.
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