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• W2071451929 startingPage "17148" @default.
• W2071451929 abstract "The doping of single-walled carbon nanotubes (SWNTs) under ultrahigh vacuum by Li atoms has been explored experimentally and theoretically. The chemical effect of Li in breaking the C−Cl bond in chloromethane has been observed. Temperature programmed desorption (TPD) experiments show that at low coverage CH3Cl is physisorbed to the undoped SWNT sample, exhibiting a desorption process near 178 K. The CH3Cl desorption peak shifts to about 240 K for lithiated SWNTs, indicating an increase in binding energy of about 0.16 eV. More importantly, the integrated intensity of the CH3Cl desorption peak is dramatically reduced in the lithiated SWNT case, and CH3, C2H6, or related species are not observed in significant quantities in the TPD experiments up to a temperature of 500 K. This strongly indicates that CH3Cl reacts on lithiated SWNTs to produce an irreversibly bound species. Products LiCl and Li2Cl2 are observed to desorb near 700 K. Density functional theory calculations present possible reaction mechanisms ..." @default.
• W2071451929 created "2016-06-24" @default.
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• W2071451929 date "2010-08-02" @default.
• W2071451929 modified "2023-09-26" @default.
• W2071451929 title "Carbon−Chlorine Bond Scission in Li-Doped Single-Walled Carbon Nanotubes: Reaction of CH₃Cl and Lithium" @default.
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• W2071451929 doi "https://doi.org/10.1021/jp103942n" @default.
• W2071451929 hasPublicationYear "2010" @default.
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