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• W2071478010 abstract "Abstract Deactivation behavior is an important topic in catalyst development. In case of methanol synthesis the conventional Cu/ZnO/Al2O3 system is commonly known to be prone to sintering, however, information about the structural development during deactivation or the sintering mechanism(s) are scarce. We present a systematic deactivation study on three different Cu/ZnO/Al2O3 catalysts which are aged under constant conditions and periodically analyzed using kinetic measurements and N2O chemisorption. A power law model for the catalyst activity with time on stream is derived. Furthermore it is found, that the presence of water provokes a steep loss in active surface area and specific activity. Also, the TEM particle size distributions generated during the aging treatment are evaluated and discussed." @default.
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• W2071478010 date "2015-08-01" @default.
• W2071478010 modified "2023-10-17" @default.
• W2071478010 title "Kinetics of deactivation on Cu/ZnO/Al2O3 methanol synthesis catalysts" @default.
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• W2071478010 doi "https://doi.org/10.1016/j.apcata.2015.06.014" @default.
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