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- W2071546727 abstract "Analytic expressions for the complex long-axis linear optical susceptibility ${ensuremath{chi}}_{mathrm{xx}}$ of parallel, noninteracting trans-polyacetylene and poly(para-phenylene) chains are obtained in terms of the band gap ${E}_{g}$ and the ensuremath{pi}-band width ${E}_{0}.$ The fact that the susceptibility expressions show identical dependence on the parameters ${E}_{g}$ and ${E}_{0}$ leads the way to a general expression for the long-axis linear optical susceptibility of conjugated polymers valid for photon energies around the band gap. The susceptibility expressions include damping and are obtained in the free-carrier dipole approximation using an analytic tight-binding derivation based on carbon $ensuremath{pi}$ electrons only. In addition to the long-axis susceptibilities, the complex short-axis susceptibility ${ensuremath{chi}}_{mathrm{yy}}$ and off-diagonal susceptibility ${ensuremath{chi}}_{mathrm{xy}}$ of trans-polyacetylene and the imaginary part of the short-axis susceptibility of poly(para-phenylene) are also derived." @default.
- W2071546727 created "2016-06-24" @default.
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- W2071546727 date "2003-02-28" @default.
- W2071546727 modified "2023-09-26" @default.
- W2071546727 title "Analytic expressions for linear optical susceptibilities of conjugated polymers" @default.
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- W2071546727 doi "https://doi.org/10.1103/physrevb.67.075206" @default.
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