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- W2071547201 startingPage "737" @default.
- W2071547201 abstract "Nuclear quadrupole resonance of ${mathrm{Cl}}^{35}$ in five hexagonal rare-earth trichlorides under hydro-static pressure up to 5ifmmodetimeselsetexttimesfi{}${10}^{3}$ kg/${mathrm{cm}}^{2}$ showed a decrease in frequency $ensuremath{nu}$ with increase in pressure. The normalized pressure coefficients ${ensuremath{nu}}_{0}^{ensuremath{-}1} {(frac{ensuremath{partial}ensuremath{nu}}{ensuremath{partial}P})}_{T}$ varied smoothly between the extremes (-5.586 ifmmodepmelsetextpmfi{} 0.020) ifmmodetimeselsetexttimesfi{} (${10}^{ensuremath{-}6}$ ${mathrm{cm}}^{2}$/kg) and (-3.855 ifmmodepmelsetextpmfi{} 0.016) ifmmodetimeselsetexttimesfi{} (${10}^{ensuremath{-}6}$ ${mathrm{cm}}^{2}$/kg) for Ce${mathrm{Cl}}_{3}$ and Gd${mathrm{Cl}}_{3}$, respectively. The negative sign suggested a model with a significant overlap contribution to the electric field gradient and a soft-sphere model was developed in analogy to the Born-Mayer model of inter-ionic repulsive forces. This model proved adequate to explain the systematic variations in ${ensuremath{nu}}_{Q}$ with compound and was consistent with the pressure dependence of $ensuremath{nu}$. The use of pressure data as a critical test for the model must await reliable compressibility data for the compounds. Pressure data for monoclinic Er${mathrm{Cl}}_{3}$ and Yb${mathrm{Cl}}_{3}$ are also presented." @default.
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- W2071547201 date "1972-08-01" @default.
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- W2071547201 title "Soft-Sphere Model for Nuclear Quadrupole Resonance: Rare-Earth Trichlorides under Hydrostatic Pressure" @default.
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- W2071547201 doi "https://doi.org/10.1103/physrevb.6.737" @default.
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