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- W2071677576 abstract "The BaTiSi 3-x Ge x O 9 crystalline phases were synthesized, and their phase-stability and photoluminescent (PL) properties were investigated. The benitoite and tetragermanate-type phases were crystallized in the range of x= 0.75-1.5 and x= 2.0-3.0, respectively. It was suggested that Ge 4+ occupies the octahedral Ti site due to the closeness of each ionic radii. The diffuse-reflection spectra revealed an increase in the oxygen-defect center by substitution of Ge in the crystalline phase. Although the BaTiSi 2.25 Ge 0.75 O 9 phase showed an efficient blue PL at room temperature, the PL intensity decreased drastically with the increasing x, and eventually the BaTiGe 3 O 9 phase indicated a very weak PL in spite of almost the same structure as benitoite, that is, the absolutely-isolated TiO 6 octahedral unit and the Ge 3 O 9 ring. It was suggested that the reduction of the PL intensity in the BaTi (Si, Ge) 3 O 9 phase was caused by the increase in the oxygen-defect center." @default.
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- W2071677576 date "2006-01-01" @default.
- W2071677576 modified "2023-09-26" @default.
- W2071677576 title "Phase-Stability and Photoluminescence of BaTi(Si, Ge)3O9" @default.
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- W2071677576 doi "https://doi.org/10.2109/jcersj.114.313" @default.
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