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• W2071728504 endingPage "146" @default.
• W2071728504 startingPage "140" @default.
• W2071728504 abstract "The electronic deactivation of the 6-oxopurine derivative hypoxanthine, its nucleoside inosine and the nucleotide inosine monophosphate have been studied by femtosecond time-resolved spectroscopy after ππ∗ photoexcitation at λ = 260 nm. The development of a highly sensitive parallel broadband (near-UV/VIS) and single-color (deep-UV) transient absorption setup enabled us to monitor the excited-state decay and the ground-state recovery dynamics in one and the same experiment. The measurements revealed similar relaxation behavior, with time constants of τ1 ≲ 0.1 ps, τ2 ≈ 0.21 ± 0.08 ps and τ3 ≈ 1.8 ± 0.4 ps, for all three investigated molecules. The observed dynamics are assumed to take place through a conical intersection involving an out-of-plane puckering mode of the six-membered ring similar to guanine." @default.
• W2071728504 created "2016-06-24" @default.
• W2071728504 creator A5028141872 @default.
• W2071728504 creator A5036000852 @default.
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• W2071728504 date "2012-05-01" @default.
• W2071728504 modified "2023-09-25" @default.
• W2071728504 title "Ultrafast electronic deactivation dynamics of the rare natural nucleobase hypoxanthine" @default.
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• W2071728504 doi "https://doi.org/10.1016/j.cplett.2012.03.106" @default.
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