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- W2071748767 endingPage "045102" @default.
- W2071748767 startingPage "045102" @default.
- W2071748767 abstract "We have studied the role of the electronic–nuclear entanglement in the emission properties of two interacting conjugated polymer chains forming an aggregate. The effect of disorder generally found in these systems is realized through a torsional degree of freedom which is responsible for a conical intersection of the adiabatic potential energy surfaces of the two excitonic states. The transition of the spectral nature of the aggregate from dimeric to monomeric form appears at the conical intersection point with vanishing entanglement of the emitting excitonic state. It is characterized by the nontrivial dependence of the emission rate for two perpendicular polarizations as a function of the torsion angle corresponding to different static disordered configurations. The exciton population dynamics shows direct connection to the entanglement evolution with the oscillations in population giving maximally entangled states as well as entanglement sudden death. A thorough analysis of the reduced densities of the nuclear degrees of freedom reveals that these extrema of entanglement can be connected to the passage of the system through the conical intersection for the range of interaction strength generally found in these systems." @default.
- W2071748767 created "2016-06-24" @default.
- W2071748767 creator A5028194950 @default.
- W2071748767 creator A5086881331 @default.
- W2071748767 date "2012-02-07" @default.
- W2071748767 modified "2023-09-24" @default.
- W2071748767 title "Electronic–nuclear entanglement in a conjugated polymer aggregate with a conical intersection: spectral signatures" @default.
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- W2071748767 doi "https://doi.org/10.1088/0953-4075/45/4/045102" @default.
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