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- W2071900190 abstract "Time-delayed four-wave mixing, using incoherent laser pulses 5 ns long and 350 AA{} wide, has been used to measure the optical phase relaxation of a large molecule (nile blue) in solution at 300 and 4.5 K. In the latter case an asymmetric response as well as a quantum beat (signaling a vibronic mode at 583 ${mathrm{cm}}^{mathrm{ensuremath{-}}1}$) is observed. Its magnitude and shape gives its electron-vibron coupling factor S=0.79 together with the homogeneous relaxation time ${mathit{T}}_{2}$=43.7 fs and the inhomogeneous relaxation time ${mathit{T}}_{2}^{mathrm{*}}$=13.3 fs (full width of 940 ${mathrm{cm}}^{mathrm{ensuremath{-}}1}$). Supporting evidence for the large value of S is presented." @default.
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- W2071900190 date "1992-07-01" @default.
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- W2071900190 title "Ultrafast relaxation and modulation in the oxazine dye nile blue" @default.
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- W2071900190 doi "https://doi.org/10.1103/physreva.46.r33" @default.
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