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- W2071957831 abstract "Abstract A PdO/Ce1−xPdxO2−δ catalyst containing surface PdOx (x = 1–2) species and Ce1−xPdxO2−δ solid solution was prepared by a solution combustion method. It was found that the surface PdOx species could be removed by nitric acid treatment. Also, partial Pd4+ cations in the CeO2 lattice migrated to the surface to form surface PdOx species after high temperature calcination (500 °C). The catalyst was tested for catalytic CO and CH4 oxidation. For CO oxidation, the specific reaction rate of the surface PdOx species ( 673 .4 μ mol CO g Pd − 1 s − 1 ) was 249 times as high as that of the Ce1−xPdxO2−δ solid solution ( 2 .7 μ mol CO g Pd − 1 s − 1 ), due to the fact that the surface PdOx species provided CO chemisorption sites. While for CH4 oxidation, the specific reaction rate of the Ce1−xPdxO2−δ solid solution ( 7 .5 μ mol CH 4 g Pd − 1 s − 1 ) was higher than that of the PdO/Ce1−xPdxO2−δ catalyst ( 2 .8 μ mol CH 4 g Pd − 1 s − 1 ), due to the covered Ce1−xPdxO2−δ surface by surface PdOx species." @default.
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- W2071957831 date "2012-05-01" @default.
- W2071957831 modified "2023-09-26" @default.
- W2071957831 title "Identification of active sites for CO and CH4 oxidation over PdO/Ce1−xPdxO2−δ catalysts" @default.
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- W2071957831 doi "https://doi.org/10.1016/j.apcatb.2012.02.036" @default.
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