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- W2072077820 abstract "Relative rotational and vibrational populations have been extracted by computer simulation of laser excited fluorescence spectra of BiF (X0+) formed in a thermal molecular beam of bismuth reacting with molecular fluorine under single-collision conditions. The observed rotational distribution is colder than the prior distribution calculated assuming three product fragments. The observed vibrational distribution is also cold, indicating that comparatively little energy is available to the ground state molecules probed. Since the dependence of the detected BiF (X0+) product on the beam time of flight points toward Bi2 as the major beam reactant, the product energy distributions presented here suggest a mechanism in which BiF (X0+), Bi (4S), and F (2P) are formed in an end-to-end attachment of Bi2 and F2. There were no indications that BiF (X0+) can be readily formed by reaction of atomic bismuth." @default.
- W2072077820 created "2016-06-24" @default.
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- W2072077820 date "1992-07-01" @default.
- W2072077820 modified "2023-10-17" @default.
- W2072077820 title "Beam‐gas study of bismuth–fluorine reactions using laser‐induced fluorescence of BiF" @default.
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- W2072077820 doi "https://doi.org/10.1063/1.463614" @default.
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