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- W2072272616 abstract "We have investigated normal-emission photoelectron spectra at various photon energies between ℏω=11.8 eV and 29.8 eV from W(110) covered with about one monolayer of dissociatively chemisorbed oxygen. As expected, O(2p)-derived bonding orbitals appear energetically below the substrate 5d-valence-band emission and these are observed at initial state energies Ei=(−5.1±0.1) eV, (−6.1±0.1) eV and (− 7.7±0.2) eV below the Fermi energy. In addition, however, drastic spectral changes are also induced in the W(5d) region and our interest is focused primarily on an understanding of the latter emission. All results clearly demonstrate its 2-dimensional character, with no detectable geometric reconstruction in the layers below. We give an interpretation in terms of emission from W(5d)–O(2p) strongly hybridized orbitals. These reside essentially in the outermost layer and are split off the bulk bands energetically by the action of the strongly oxygen-modified surface potential. By checking for intensity variations with ℏω the overlayer orbitals can be identified in terms of their parent bulk bands." @default.
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- W2072272616 date "1999-10-01" @default.
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- W2072272616 title "Normal-emission photoelectron studies of the W(110)(1×1)O surface" @default.
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- W2072272616 doi "https://doi.org/10.1016/s0039-6028(99)00796-7" @default.
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