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• W2072357245 abstract "It was commonly accepted that alkanethiols (C2H2n + 1SH) self assemble on Au(111) into the (√3 × √3)R30 structure by chemisorption of the sulfur atoms to the three-fold hollow sites. However, the observation of (p × √3) structures and evidence for dimerized sulfurs on the substrate have questioned this model. We have imaged alkanethiols on Au(111) for 4 ≤ n ≤ 8 by scanning tunneling microscopy under ambient conditions. We found (p × √3) structures for n ≤ 6 and the (√3 × √3)R30 structure for n ≥ 7 both for high densities of (22 ± 2) Å2 per molecule indicating a dependence of structure on chain-length. We can describe our observations by two distinct crystalline phases of dimerized thiol molecules." @default.
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• W2072357245 date "1998-03-01" @default.
• W2072357245 modified "2023-09-25" @default.
• W2072357245 title "Chain-length-dependent structure of alkanethiols forming dimers on Au(111)" @default.
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• W2072357245 doi "https://doi.org/10.1016/s0039-6028(97)00829-7" @default.
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