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- W2072461608 abstract "Abstract By making use of iron electrodes the thermoelectric power has been measured for ferrous oxide and ferrous oxide + silicate mixtures in the liquid and solid state and for molten ferrous oxide + calcium oxide mixtures. The measurements are made with the samples suspended between iron electrodes in the temperature range 1150–1470°C. The θ3, the thermoelectric power corrected with respect to the effect of iron electrode shows −12 ~ 23 μV/deg for the ferrous oxide, 0 ~ −134 μV/deg for the ferrous oxide containing from 9.6 to 33.2% silica at 1400°C, and positive values for the ferrous oxide + calcium oxide mixtures. These results are interpreted in terms of equations derived from non-equilibrium thermodynamics, since in this non-stoichiometric compounds the concentration of charge carriers (or positive hole) depends upon local temperature and the heterogeneous thermoelectric power is not negligible compared with the homogeneous part. In particular, it is pointed out that the heat of transport of the charge carrier may be practically equal to the heat of activation in the ‘FeO’ system and the ‘FeO’ + SiO 2 (~30%) mixtures and that the composition dependence of the free volume (or vibrational frequency) of ferrous ion may be important to interpret the data in the ‘FeO’~SiO2 mixtures." @default.
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- W2072461608 date "1968-09-01" @default.
- W2072461608 modified "2023-09-27" @default.
- W2072461608 title "On the thermoelectric power of the system ‘FeO’, ‘FeO’-SiO2 and ‘FeO’-CaO" @default.
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