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• W2072614818 abstract "Lithium sulfide is a promising cathode material for high-energy lithium ion batteries because, unlike elemental sulfur, it obviates the need for metallic lithium anodes. Like elemental sulfur, however, a successful lithium sulfide cathode requires an inherent mechanism for preventing lithium polysulfide dissolution and shuttling during electrochemical cycling. A new scheme is proposed to create composites based on lithium sulfide uniformly dispersed in a carbon host, which serve to sequester polysulfides. The synthesis methodology makes use of interactions between lithium ions in solution and nitrile groups uniformly distributed along the chain backbone of a polymer precursor (e.g., polyacrylonitrile), to control the distribution of lithium sulfide in the host material. The Li(2)S-carbon composites obtained by carbonizing the precursor are evaluated as cathode materials in a half-cell lithium battery, and are shown to yield high galvanic charge/discharge capacities and excellent Coulombic efficiency, demonstrating the effectiveness of the architecture in homogeneously distributing Li(2)S and in sequestering lithium polysulfides." @default.
• W2072614818 created "2016-06-24" @default.
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• W2072614818 date "2012-12-28" @default.
• W2072614818 modified "2023-10-14" @default.
• W2072614818 title "Lithium–Sulfur Battery Cathode Enabled by Lithium–Nitrile Interaction" @default.
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• W2072614818 doi "https://doi.org/10.1021/ja309435f" @default.
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