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- W2072649215 abstract "The effect of soluble silicate on the sorption of U(VI) to γ-Al2O3 was investigated by batch experiments and extended X-ray absorption fine structure (EXAFS) method. The presence of silicate enhanced the sorption of U(VI) on γ-Al2O3 surface and the sorption was attributed to inner-sphere surface complexation. The structure of the adsorbed U(VI) and silicate on γ-Al2O3 was investigated in the analysis of EXAFS spectra. The fitting of the experimental EXAFS data was obtained by including two uranium coordination shells with 2 axial (Oax) and 5 equatorial (Oeq) oxygen atoms at 1.79 ± 0.02 and 2.43 ± 0.02 Å, respectively, and the third coordination shells with Al atom at ∼3.35 Å. Silicate contributed to the formation of ternary inner-sphere surface complexes, acting as “bridge” between U(VI) and γ-Al2O3 and enhanced the sorption of U(VI). The observations suggested that the interactions between U(VI) and silicate were important in controlling U(VI) retention." @default.
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- W2072649215 date "2015-06-01" @default.
- W2072649215 modified "2023-10-17" @default.
- W2072649215 title "Effect of silicate on U(VI) sorption to γ-Al2O3: Batch and EXAFS studies" @default.
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- W2072649215 doi "https://doi.org/10.1016/j.cej.2015.01.121" @default.
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