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- W2072880565 abstract "Abstract The oxide ion conduction mechanism was clarified for high purity RE 9.33 (SiO 4 ) 6 O 2 and Sr 2 RE 8 (SiO 4 ) 6 O 2 (RE = La and Nd) by Rietveld and maximum entropy method (MEM) analysis using neutron powder diffraction data collected at room temperature. All the compounds had an apatite-type structure in the space group P6 3 /m. Neither site splitting nor interstitial sites of the oxide ion was observed. RE 9.33 (SiO 4 ) 6 O 2 had cation vacancies only at the 4 f site. In Sr 2 RE 8 (SiO 4 ) 6 O 2 , the 4 f sites were fully occupied by strontium and rare earths with a molar ratio of 1 : 1. Also, in RE 9.33 (SiO 4 ) 6 O 2 , the oxide ion at the hexagonal channel site had a large displacement along the c -axis. This large displacement is induced by cooperative rotation of SiO 4 tetrahedra around rare earths at the 4 f site through oxide ion polyhedra around another rare earth at the 6 h site. The displacement, enhanced by a vacancy in the 4 f site, is directly related to oxide ion conduction in RE 9.33 (SiO 4 ) 6 O 2 ." @default.
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- W2072880565 date "2006-01-01" @default.
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- W2072880565 title "Oxide ion conduction mechanism in RE9.33(SiO4)6O2 and Sr2RE8(SiO4)6O2 (RE=La, Nd) from neutron powder diffraction" @default.
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- W2072880565 doi "https://doi.org/10.1016/j.ssi.2005.09.015" @default.
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