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- W2073042337 abstract "Microcalorimetric measurements were carried out to explain reactions of H+>OH− on the surface of three different groups of minerals: oxides, salt-type minerals, and kaolinite and feldspar. The results were compared to those of H+>OH− adsorption density measurements and to the isoelectric points, obtained from electrophoretic mobility measurements at different pH. In oxides with H+>OH− as predominant potential-determining ions, a good agreement was found between results of equiadsorption point measurements obtained by both methods. In all oxides studied, the adsorption of H+ and OH− proceeded exothermically. In minerals of the remaining two groups, except for barite and fluorite, the reaction heats of H+ with the surface were much higher than those in oxides. Since the H+>OH− adsorption densities are much lower, the heat effect is mostly due to a dissolution of the salt lattice and hydration of free lattice ions. Barite and fluorite showed an anomalous behavior, the cause of which is discussed. Calorimetric measurements on kaolinite confirmed that the edge share of the whole kaolinite surface (10%) is responsible for the adsorption of H+ and OH−." @default.
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- W2073042337 date "1988-03-01" @default.
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- W2073042337 title "Exchange enthalpies of H+ and OH− adsorption on minerals with different characters of potential-determining ions" @default.
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- W2073042337 doi "https://doi.org/10.1016/0021-9797(88)90300-1" @default.
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