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• W2073055013 startingPage "9808" @default.
• W2073055013 abstract "7Li NMR spectroscopy and relaxometry are exploited to obtain structural and dynamical information within heterogeneous systems resulting from aqueous dispersion of clay platelets. In addition to the specific orientation of the clay platelets detected by the splitting of the 7Li resonance line, multiquantum relaxation measurements are used to determine the relative contributions from the quadrupolar and dipolar relaxation mechanisms responsible for the detected broadening of the 7Li resonance line. Intrinsic spectral densities are further extracted from the variation of these apparent relaxation rates as a function of the orientation of the clay sediment within the static magnetic field. A semiquantitative interpretation of the intrinsic quadrupolar and dipolar relaxation behavior is performed by a multiscale modeling of the Li+ ions’ diffusion in relation to the structure of the clay dispersions. Equivalent structural and dynamical investigations can be performed within a broad class of material containing electrically charged solid/liquid interfaces by exploiting the sensitivity of 7Li NMR spectroscopy." @default.
• W2073055013 created "2016-06-24" @default.
• W2073055013 creator A5005319370 @default.
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• W2073055013 date "2008-06-11" @default.
• W2073055013 modified "2023-09-25" @default.
• W2073055013 title "⁷Li NMR Spectroscopy and Multiquantum Relaxation as a Probe of the Microstructure and Dynamics of Confined Li⁺ Cations: An Application to Dense Clay Sediments" @default.
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• W2073055013 doi "https://doi.org/10.1021/jp8010348" @default.
• W2073055013 hasPublicationYear "2008" @default.
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