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• W2073158470 endingPage "124801" @default.
• W2073158470 startingPage "124801" @default.
• W2073158470 abstract "Quantum dynamics calculations via the local reflection matrix method are performed to investigate the effects of the vibration and initial translational energy on the dissociative adsorption of H2 approaching a defective Pt(111) surface at different incident angles and adsorption sites. The sticking probability plot for H2 incident on the top site at 15° shows that as the translational energy is increased, the probability rapidly rises to unity which suggests that H2 is easily adsorbed on the Pt surface. The plot also shows that even though the adsorption process is non-activated, there is a probability that H2 will not be adsorbed on the Pt surface at low translational energies due to quantum mechanical effects. For the rest of the configurations, an S-shaped region is observed in the plots suggesting an activated adsorption process. The plots show that when the initial translational energy (Et) is less that the barrier, H2 sticks to the Pt surface by tunneling through the barrier and when Et is greater ..." @default.
• W2073158470 created "2016-06-24" @default.
• W2073158470 creator A5022197171 @default.
• W2073158470 creator A5023399092 @default.
• W2073158470 creator A5070852791 @default.
• W2073158470 date "2014-12-15" @default.
• W2073158470 modified "2023-09-23" @default.
• W2073158470 title "Quantum Dynamics Study on the Effects of Vibration, Translational Energy and Incident Angle on H2 Adsorption on a Defective Pt(111) Surface" @default.
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• W2073158470 doi "https://doi.org/10.7566/jpsj.83.124801" @default.
• W2073158470 hasPublicationYear "2014" @default.
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