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- W2073179660 abstract "Control of the torsional angles of nonrigid molecules is key for the development of emerging areas like molecular electronics and nanotechnology. Based on a rigorous calculation of the rotation-torsion-Stark energy levels of nonrigid biphenyl-like molecules, we show that, unlike previously believed, instantaneous rotation-torsion-Stark eigenstates of such molecules, interacting with a strong laser field, present a large degree of delocalization in the torsional coordinate even for the lowest energy states. This is due to a strong coupling between overall rotation and torsion leading to a breakdown of the torsional alignment. Thus, adiabatic control of changes on the planarity of this kind of molecule is essentially impossible unless the temperature is on the order of a few Kelvin." @default.
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- W2073179660 date "2011-09-08" @default.
- W2073179660 modified "2023-09-30" @default.
- W2073179660 title "Rotation-Induced Breakdown of Torsional Quantum Control" @default.
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- W2073179660 doi "https://doi.org/10.1103/physrevlett.107.113004" @default.
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