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• W2073208997 endingPage "1071" @default.
• W2073208997 startingPage "1069" @default.
• W2073208997 abstract "The kinetics of photoinduced electron-transfer (ET) reactions have been measured in a series of synthetic donor-acceptor complexes. The electron donors are singlet or triplet excited iridium(I) dimers (Ir(2)), and the acceptors are N-alkylpyridinium groups covalently bound to phosphinite ligands on the Ir(2) core. Rate constants for excited-state ET range from 3.5 x 10(6) to 1.1 x 10(11) per second, and thermal back ET (pyridinium radical to Ir(2)(+)) rates vary from 2.0 x 10(10) to 6.7 x 10(7) per second. The variation of these rates with driving force is in remarkably good agreement with the Marcus theory prediction of a Gaussian free-energy dependence." @default.
• W2073208997 created "2016-06-24" @default.
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• W2073208997 date "1990-03-02" @default.
• W2073208997 modified "2023-10-14" @default.
• W2073208997 title "Gaussian Free-Energy Dependence of Electron-Transfer Rates in Iridium Complexes" @default.
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• W2073208997 doi "https://doi.org/10.1126/science.247.4946.1069" @default.
• W2073208997 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/17800065" @default.
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