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• W2073344706 abstract "Abstract Highly dispersed FeMn bimetallic particles were obtained on a high-surface-area amorphous carbon black support using FeMn and KFeMn carbonyl clusters. These catalysts were characterized by hydrogen adsorption and by CO chemisorption at 195 and 300 K, and their kinetic behavior for CO hydrogenation was studied at 1 atm in a differential, plug-flow microreactor. The K-promoted clusters with stoichiometries of KMnFe and KMnFe2 gave 85–90 wt% ethylene, propylene, and butene with methane as the only other detectable hydrocarbon product. The KFe3 cluster also had a high selectivity to olefins but showed somewhat more chain growth. The nonpromoted MnFe catalysts with Fe Mn = 2 , prepared from either stoichiometric mixed-metal carbonyl clusters or coimpregnation of the separate Fe and Mn carbonyl clusters, also had a high selectivity to light olefins; however, this selectivity was strongly dependent upon the pretreatment. The properties of the FeMn clusters without K is consistent with a proposed model in which a surface spinel, (Fel-yMny)3O4, plays a principal role in providing high selectivity to light olefins." @default.
• W2073344706 created "2016-06-24" @default.
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• W2073344706 date "1987-02-01" @default.
• W2073344706 modified "2023-09-26" @default.
• W2073344706 title "Carbon-supported Fe$z.sbnd;Mn and K$z.sbnd;Fe$z.sbnd;Mn clusters for the synthesis of C2$z.sbnd;C4 olefins from CO and H2 I. Chemisorption and catalytic behavior" @default.
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• W2073344706 doi "https://doi.org/10.1016/0021-9517(87)90136-9" @default.
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