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- W2073427375 abstract "The π electron system of the basic indigo chromophore can formally be obtained by joining two identical fragments; the coupling of two radical centres thus affords one bonding and one antibonding π MO, which form the HOMO and the LUMO of the system. A small HOMO-LUMO splitting and thus a long-wavelength absorption result from a pronounced delocalization of the unpaired electron in the radical fragments due to the captodative radical stabilization. Results of SCF calculations within the π electron approximation confirm these ideas." @default.
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- W2073427375 date "1982-04-01" @default.
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- W2073427375 title "The origin of the colour of indigo dyes" @default.
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- W2073427375 doi "https://doi.org/10.1016/0143-7208(82)80025-9" @default.
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