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• W2073643874 abstract "We show that the equilibrium size of single-layer shells composed of polyoxometalate macroions is inversely proportional to the dielectric constant of the medium in which they are dispersed. This behavior is consistent with a stabilization mechanism based on Coulomb repulsion combined with charge regulation. We estimate the cohesive energy per bond between macroions on the shells to be approximately -6kT. This number is extracted from analysis based on a charge regulation model in combination with a model for defects on a sphere. The value of the cohesive bond energy is in agreement with the model-independent critical aggregate concentration. This observation points to a new class of thermodynamically stable shell-like objects. We point out the possible relevance our findings have for certain surfactant systems." @default.
• W2073643874 created "2016-06-24" @default.
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• W2073643874 date "2007-08-08" @default.
• W2073643874 modified "2023-10-18" @default.
• W2073643874 title "Charge Regulation as a Stabilization Mechanism for Shell-Like Assemblies of Polyoxometalates" @default.
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• W2073643874 doi "https://doi.org/10.1103/physrevlett.99.066104" @default.
• W2073643874 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/17930844" @default.
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