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• W2073668668 endingPage "371" @default.
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• W2073668668 abstract "A short review of the field of collisions of slow cluster ions with surfaces is presented. The main subject of the paper is a survey of results of a series of studies on slow cluster ion collisions with surfaces carried out in Innsbruck. In these studies the incident ions were fullerene multiply-charged ions and small cluster ions of polyatomic molecules (acetone and acetonitrile radical cations, protonated ethanol, clustered by 2–4 monomer molecules). For collisions of multiply-charged fullerene cations C60z+ (z from 1 to 5, incident energies 100–500 eV) only singly-charged product ions were observed which were formed by sequential loss of C2 units. The effect of multiple-charge of the projectile on its fragmentation was less pronounced than expected from a full conversion of electronic energy gained in the surface neutralization process. Fragmentation upon surface collision excitation of acetone, acetonitrile and protonated ethanol cluster ions (incident energies 10–80 eV) was found to follow the unimolecular dissociation kinetics. Formation of protonated monomers in collisions of acetone and acetonitrile stoechiometric clusters resulted both from an intra-cluster reaction and from a reaction of the monomer product ion with the surface hydrogen; it could be rationalized using the double-well potential model. Incident energy dependence of relative abundance of dissociation products from surface collisions of protonated ethanol trimers, dimers and monomers could be mutually rationalized, if the fraction of energy transformed in the surface collision into internal energy was related to one internal degree of freedom. A diagram resembling a break-down pattern of the projectile ion was obtained in this way. All internal degrees of freedom of the projectile ion seemed to be involved in the unimolecular dissociation kinetics." @default.
• W2073668668 created "2016-06-24" @default.
• W2073668668 creator A5078657567 @default.
• W2073668668 date "2004-04-01" @default.
• W2073668668 modified "2023-10-10" @default.
• W2073668668 title "Surface collisions of small cluster ions at incident energies 10–102eV" @default.
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• W2073668668 doi "https://doi.org/10.1016/j.ijms.2004.01.011" @default.
• W2073668668 hasPublicationYear "2004" @default.
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