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- W2073680905 abstract "Iron oxide modified with single- or double-metal additives (Cr, Ni, Zr, Ag, Mo, Mo-Cr, Mo-Ni, Mo-Zr and Mo-Ag), which can store and supply pure hydrogen by reduction of iron oxide with hydrogen and subsequent oxidation of reduced iron oxide with steam (Fe{sub 3}O{sub 4} (initial Fe{sub 2}O{sub 3})+4H{sub 2}reversible3Fe+4H{sub 2}O), were prepared by impregnation. Effects of various metal additives in the samples on hydrogen production were investigated by the above-repeated redox. All the samples with Mo additive exhibited a better redox performance than those without Mo, and the Mo-Zr additive in iron oxide was the best effective one enhancing hydrogen production from water decomposition. For Fe{sub 2}O{sub 3}-Mo-Zr, the average H{sub 2} production temperature could be significantly decreased to 276 deg. C, the average H{sub 2} formation rate could be increased to 360.9-461.1 {mu}mol min{sup -1} Fe-g{sup -1} at operating temperature of 300 deg. C and the average storage capacity was up to 4.73 wt% in four cycles, an amount close to the IEA target. - Graphical abstract: Mo+Zr additive has the best modified effect on improving the redox performances of Fe{sub 2}O{sub 3}:H{sub 2} producing temperature of 276 deg. C and hydrogen storage capacity of 4.73 wt%." @default.
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- W2073680905 date "2010-05-01" @default.
- W2073680905 modified "2023-09-23" @default.
- W2073680905 title "Hydrogen production from water decomposition by redox of Fe2O3 modified with single- or double-metal additives" @default.
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- W2073680905 doi "https://doi.org/10.1016/j.jssc.2010.03.017" @default.
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