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- W2073973145 abstract "The electronic structure of BeAl was investigated by laser induced fluorescence and resonance enhanced multiphoton ionization spectroscopy. BeAl was formed by pulsed laser ablation of a Be/Al alloy in the presence of helium carrier gas, followed by a free jet expansion into vacuum. In agreement with recent ab initio studies, the molecule was found to have a 2Π1/2 ground state. Transitions to two low lying electronic states, (2)2Π1/2(v′) ← X 2Π1/2 (v″ = 0) and (1)2Δ(v′) ← X 2Π1/2 (v″ = 0,1), were observed and rotationally analyzed. An additional band system, identified as (4)2Σ+(v′) ← X 2Π1/2, was found in the 28 000–30 100 cm−1 energy range. This transition exhibited an unusual pattern of vibrational levels resulting from an avoided crossing with the (5)2Σ+ electronic state. New multi-reference configuration interaction calculations were carried out to facilitate the interpretation of the UV bands." @default.
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- W2073973145 date "2008-01-01" @default.
- W2073973145 modified "2023-09-25" @default.
- W2073973145 title "Experimental and theoretical study of the electronic spectrum of BeAl" @default.
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- W2073973145 doi "https://doi.org/10.1039/b806879h" @default.
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