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• W2074066768 abstract "Es wird über die Synthese und Eigenschaften der Methyllithium-Komplexe von Nickel(0) (n-Donor)m(LiCH3)Ni0(π-Ligand)n On the Lewis Acidity of Nickel(0), I. Methyllithium Complexes of Nickel(0) The synthesis and properties of the methyllithium complexes of nickel(0) of the type (n-Donor)m-(LiCH3)Ni0(π-Ligand)n (1a–c, 16a–c, 20a–c) [n-Donor = chelating amine or THF; π-Ligand = CDT, ethene, or CO] are described. The structure of (PMDTA)(LiCH3)Ni(C2H4)2 (1b) has been determined by X-ray crystallography. — In these ate complexes, a carbanionic methyl group is σ-bonded to a nickel atom, the acceptor strength of which depend on the π-ligands. The chemical and spectroscopic properties indicate that the NiCH3 bond in the carbonyl complex is largely covalent whereas in the CDT and ethene compounds it is more polar. The CDT complex is thermolabile in solution. The findings are in agreement with the following series of increasing acceptor strength: Ni(CDT) < Ni(C2H4)2 < Ni(CO)3." @default.
• W2074066768 created "2016-06-24" @default.
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• W2074066768 date "1985-01-01" @default.
• W2074066768 modified "2023-10-02" @default.
• W2074066768 title "Zur Lewis‐Acidität von Nickel(0), I. Methyllithium‐Komplexe von Nickel(0)" @default.
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• W2074066768 doi "https://doi.org/10.1002/cber.19851180126" @default.
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