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• W2074099340 startingPage "4770" @default.
• W2074099340 abstract "Photoelectron spectroscopy with monochromatic synchrotron radiation (100--115 eV) is used to study the silicon 2p excitation and ionization in the silane molecule. Valence main bands and satellites are observed when ${mathrm{SiH}}_{4}$ is excited below the Si 2p edge and off resonance. Auger lines are seen for excitation energies above the edge. The excitation of a core electron into the lowest antibonding molecular orbital results in dramatic changes in the spectrum. In addition to autoionization and resonant Auger processes, which lead to ${mathrm{SiH}}_{4}$ with one-hole and two-hole--one-particle (or multiple-hole) excited configurations, respectively, an unexpected relaxation pathway due to the purely repulsive character of the core-excited state is proposed to explain the existence of very low binding energy resonating lines. It consists of a very fast dissociation into ${mathrm{SiH}}_{3}$${mathrm{}}^{mathrm{*}}$+H followed by autoionization of the core-excited ${mathrm{SiH}}_{3}$${mathrm{}}^{mathrm{*}}$ fragments." @default.
• W2074099340 created "2016-06-24" @default.
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• W2074099340 date "1986-12-01" @default.
• W2074099340 modified "2023-09-23" @default.
• W2074099340 title "Relaxation processes of resonances in<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=normal>SiH</mml:mi></mml:mrow><mml:mrow><mml:mn>4</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>in the vicinity of the silicon 2<i>p</i>threshold" @default.
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• W2074099340 doi "https://doi.org/10.1103/physreva.34.4770" @default.
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