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- W2074163078 abstract "Essentially all undoped cuprates exhibit a quasiplanar, fourfold Cu-O coordination responsible for the magnetically active antibonding $3{d}_{{x}^{2}ensuremath{-}{y}^{2}}$ like state. Here, we present an electronic structure study for ${mathrm{CuSb}}_{2}{mathrm{O}}_{6}$ that reveals, in contrast, a half-filled $3{d}_{3{z}^{2}ensuremath{-}{r}^{2}}$ orbital. This hitherto unobserved ground state originates from a competition of in- and out-of-plaquette orbitals where the strong Coulomb repulsion drives the surprising and unique orbital ordering. This, in turn, gives rise to an unexpected quasi-one-dimensional magnetic behavior. Our results provide a consistent explanation of recent thermodynamical and neutron diffraction measurements." @default.
- W2074163078 created "2016-06-24" @default.
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- W2074163078 date "2008-06-09" @default.
- W2074163078 modified "2023-09-27" @default.
- W2074163078 title "Quasi-One-Dimensional Magnetism Driven by Unusual Orbital Ordering in<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:msub><mml:mi>CuSb</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi mathvariant=normal>O</mml:mi><mml:mn>6</mml:mn></mml:msub></mml:math>" @default.
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- W2074163078 doi "https://doi.org/10.1103/physrevlett.100.237202" @default.
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