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• W2074319610 abstract "Novel amylose and cellulose derivatives bearing pyridine N-oxide groups were synthesized, and their performance as asymmetric organocatalysts was investigated. The amylose derivatives bearing 3-pyridyl N-oxide groups enantioselectively catalyzed the allylation of benzaldehyde by allyltrichlorosilane with different enantiomeric excesses (ee; 13–32% ee), depending on the degree of substitution of the pyridine N-oxide. In contrast, the corresponding cellulose derivatives showed the opposite enantioselectivity with much lower ee (2–11% ee). These results suggest that the higher-order structures of polysaccharides play an important role in the enantioselective allylation of benzaldehyde." @default.
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• W2074319610 date "2011-10-01" @default.
• W2074319610 modified "2023-10-10" @default.
• W2074319610 title "Synthesis of polysaccharide derivatives bearing pyridine N-oxide groups and their use as asymmetric organocatalysts" @default.
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• W2074319610 doi "https://doi.org/10.1016/j.reactfunctpolym.2011.07.010" @default.
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