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- W2074403713 abstract "The molecular structure of aluminium and iron(III) complexes with 3-phenyl and 3-(4-pyridyl) (HL) substituted acetylacetonate ligands is appreciably distorted. For AlL3 and FeL3 this shows that the orientation of the side pyridyl-N donor atoms lone pairs is about 90 and 135° which favours the assembly of heterobimetallic square patterns in Al(Fe)L3 complexes with metal ions. This was employed for the modular construction of semi-regular heterobimetallic networks, in which the pyridyldiketonate ligands bridge pairs of Fe(Al)/Cd(Co) metal ions and support the structure of 1D and 2D coordination polymers. The unprecedented 2D structure of [Cd{AlL3}(CH3OH){NO3}2]·2CHCl3 and Cd{AlL3}(CH3OH)Br2]·2CHCl3·2CH3OH is based upon plane tiling by a set of heterobimetallic squares and octagons, while [Cd{FeL3}2(NO3)2]·2H2O and [Co{AlL3}2Cl2]·4CHCl3·2CH3OH are 1D polymers and exist as chains of heterobimetallic squares sharing opposite vertices." @default.
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- W2074403713 date "2004-01-01" @default.
- W2074403713 modified "2023-10-12" @default.
- W2074403713 title "Extended coordination frameworks incorporating heterobimetallic squares" @default.
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- W2074403713 doi "https://doi.org/10.1039/b407244h" @default.
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