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- W2074513963 abstract "The gas phase hydrogenation of acrolein over 7.5% Ag/SiO2 has been studied in a broad pressure range from 7.5 mbar to 20 bar. Higher pressures favour the formation of allyl alcohol (selectivities up to 42%), whereas at low pressures propionaldehyde is by far the main product. In situ-XAS has been performed at 7.5 mbar in order to gain insight into the interaction of acrolein with Ag(1 1 1). Hydrogenated propionaldehyde-like surface species could be detected which orientated parallel to the surface. The observed intermediate correlates perfectly with the online catalytic data." @default.
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- W2074513963 date "2005-05-01" @default.
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- W2074513963 title "In situ-XAS and catalytic study of acrolein hydrogenation over silver catalyst: Control of intramolecular selectivity by the pressure" @default.
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- W2074513963 doi "https://doi.org/10.1016/j.catcom.2005.02.013" @default.
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