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• W2074607789 abstract "Self-assembled monolayers (SAMs) of C6H5–C≡C–C6H4–C≡C–C6H4SH (1) on Au(111) and Ag(111) exhibit electrical rectifying behavior when probed by the scanning tunneling microscope whereas SAMs derived from decanethiol, benzenethiol and 4-phenylethynylbenzenethiol do not. We suggest that rectification arises from the conjugated length of the molecular framework of 1 and an increase of the donor character of the sulfur atom to this system upon adsorption to the metal. This is supported by surface second-harmonic generation measurements which show a significantly larger second order optical nonlinearity of SAMs of 1 compared to the other systems." @default.
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• W2074607789 date "1997-03-22" @default.
• W2074607789 modified "2023-09-25" @default.
• W2074607789 title "Self-assembled molecular rectifiers" @default.
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• W2074607789 doi "https://doi.org/10.1063/1.473523" @default.
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