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- W2074717070 abstract "The usual approach to second harmonic generation (SHG) is based on low-order pertubation theory and neglects the changes in the electronic states that are induced by the exciting beam. To see whathappens in this approximation fails we propose a new formalism, based on the method of excitation amplitudes, to set up a theory of the SHG response and other inelastic light scattering phenomena. We develop the quantum theory in the dipole approximation and show that the inclusion of electron-photon coupling to all others leads to new features. Strong exciting fields produce a nonnegligible SHG response in highly polarisable centro-symmetric systems, and the emitted spectrum shows a dynamical Stark effect." @default.
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- W2074717070 date "1993-09-01" @default.
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- W2074717070 title "Many-photon effects in inelastic light scattering" @default.
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- W2074717070 doi "https://doi.org/10.1016/0375-9601(93)90294-a" @default.
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