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- W2074861646 abstract "We report the formation of monomeric and J-aggregated 1,1‘-diethyl-3,3‘-di(4-sulfobutyl)-5,5‘,6,6‘-tetrachlorobenzimidazolocarbocyanine (referred to as TDBC) encapsulated within a silicate mesostructure, specifically SBA-15, under different pH conditions. To facilitate incorporation of TDBC, it was necessary to functionalize the interface of the synthesized SBA-15 for proper guest−host electrostatic interaction between the anionic dye and the inner core surface charge, through use of a silylation reagent, (aminopropyl)triethoxysilane, which at high pH values results in formation of −NH3+ surface species. XRD, UV-vis absorption and fluorescence measurements are used as spectroscopic tools to characterize SBA-15 host samples as well as composites consisting of the host and encapsulated molecules. J-aggregated TDBC occluded within SBA-15 represents a robust, new superradiant fluorescent nanomaterial." @default.
- W2074861646 created "2016-06-24" @default.
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- W2074861646 date "2002-01-29" @default.
- W2074861646 modified "2023-09-28" @default.
- W2074861646 title "Absorption and Exciton Emission by an Aggregated Cyanine Dye Occluded within Mesoporous SBA-15" @default.
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- W2074861646 doi "https://doi.org/10.1021/jp013042y" @default.
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