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• W2074916400 startingPage "2471" @default.
• W2074916400 abstract "Two new ruthenium(II) polypyridyl dimers containing the large planar aromatic bridging ligands 9,11,20,22-tetraazatetrapyrido[3,2-a:2‘3‘-c:3‘ ‘,2‘ ‘-l:2‘ ‘‘,3‘ ‘‘-n]pentacene (tatpp) and 9,11,20,22-tetraazatetrapyrido[3,2-a:2‘3‘-c:3‘ ‘,2‘ ‘-l:2‘ ‘‘,3‘ ‘‘-n]pentacene-10,21-quinone (tatpq) have been synthesized and characterized by 1H and 13C NMR, MALDI mass spectrometry, and elemental analyses. The electronic properties (UV−vis, redox, photophysical) of these dimers are analyzed in the context of orbital calculations (PM3 level) on the bridging ligands. A localized orbital model is proposed in which low-lying acceptor orbitals on the center portion of the ligands effectively quench the Ru(II)-based MLCT emission via a mechanism that can be viewed as intramolecular electron transfer to specific subunits of the bridges." @default.
• W2074916400 created "2016-06-24" @default.
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• W2074916400 date "2002-03-30" @default.
• W2074916400 modified "2023-09-26" @default.
• W2074916400 title "Dinuclear Ruthenium(II) Polypyridyl Complexes Containing Large, Redox-Active, Aromatic Bridging Ligands: Synthesis, Characterization, and Intramolecular Quenching of MLCT Excited States" @default.
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• W2074916400 doi "https://doi.org/10.1021/ic011028u" @default.
• W2074916400 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/11978115" @default.
• W2074916400 hasPublicationYear "2002" @default.
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